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Journal Articles

Quantitative analysis of microstructure evolution, stress partitioning and thermodynamics in the dynamic transformation of Fe-14Ni alloy

Li, L.*; Miyamoto, Goro*; Zhang, Y.*; Li, M.*; Morooka, Satoshi; Oikawa, Katsunari*; Tomota, Yo*; Furuhara, Tadashi*

Journal of Materials Science & Technology, 184, p.221 - 234, 2024/06

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Validation of the hybrid turbulence model in detailed thermal-hydraulic analysis code SPIRAL for fuel assembly using sodium experiments data of 37-pin bundles

Yoshikawa, Ryuji; Imai, Yasutomo*; Kikuchi, Norihiro; Tanaka, Masaaki; Ohshima, Hiroyuki

Nuclear Technology, 210(5), p.814 - 835, 2024/05

In the study of safety enhancement on advanced sodium-cooled fast reactor, it is essential to clarify the thermal-hydraulics under various operation conditions in a fuel assembly (FA) with the wire-wrapped fuel pins to assess the structural integrity of the fuel pin. A finite element thermal-hydraulics analysis code named SPIRAL has been developed to analyze the detailed thermal-hydraulics phenomena in a FA. In this study, the numerical simulations of the 37-pin bundle sodium experiments at different Re number conditions, including a transitional condition between laminar and turbulent flows and turbulent flow conditions, were performed to validate the hybrid turbulence model equipped in SPIRAL. The temperature distributions predicted by SPIRAL was consistent with those measured in the experiments. Through the validation study, the applicability of the hybrid turbulence model in SPIRAL to thermal-hydraulic evaluation of sodium-cooled FA in the wide range of Re number was confirmed.

Journal Articles

Background and understanding on ALPS treated water discharge to the sea

Terasaka, Yuta; Iimoto, Takeshi*; Saso, Michitaka*; Fujita, Reiko*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 66(4), p.203 - 207, 2024/04

no abstracts in English

JAEA Reports

Assessment of probability of aircraft crashes for Nuclear Science Research Institute

Kamikawa, Yutaka; Suzuki, Makoto; Agake, Toshiki; Murakami, Takahiko; Morita, Yusuke; Shiina, Hidenori; Fukushima, Manabu; Hirane, Nobuhiko; Ouchi, Yasuhiro

JAEA-Technology 2023-030, 57 Pages, 2024/03

JAEA-Technology-2023-030.pdf:1.93MB

Owing to the publication of the latest data about aircraft crashes by Nuclear Regulation Authority (NRA), it was necessary to re-evaluate the probabilities of aircraft crashes for Nuclear Science Research Institute (NSRI). By using of the assessment method provided in "Regulatory Guide of the Assessment Standard for Probability of Airplane Crash on a Nuclear Power Reactor Facility", we re-evaluated the probabilities of aircraft crashes against the nuclear facilities in NSRI. As a result of the evaluations, the sum of the probabilities of aircraft crashes against Waste Treatment Facilities (maximum probability among all nuclear facilities in NSRI) is 5.68$$times$$10$$^{-8}$$ (times/(reactor $$cdot$$ year)) which is lower than 10$$^{-7}$$ (times/(reactor $$cdot$$ year)) that is the assessment criterion whether aircraft crashes is considered to be "anticipated external human induced events" in design basis or not.

JAEA Reports

Investigations on distribution of radioactive substances owing to the Fukushima Daiichi Nuclear Power Station Accident in the fiscal year 2022 (Contract research)

Group for Fukushima Mapping Project

JAEA-Technology 2023-024, 176 Pages, 2024/03

JAEA-Technology-2023-024.pdf:22.16MB

This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2022. Car-borne surveys, a measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create their distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. The range of fluctuation of past tritium concentration data in seawater was determined, and the causes of the fluctuation were discussed. Monitoring data in coastal area performed in 2022 owing to the comprehensive radiation monitoring plan was summarized, and temporal changes in cesium-137 were analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated air dose rate distribution data acquired through surveys such as car-borne and walk surveys with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2022 were published on the "Database for Radioactive Substance Monitoring Data", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.

JAEA Reports

Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Fukushima University*

JAEA-Review 2023-024, 109 Pages, 2024/03

JAEA-Review-2023-024.pdf:5.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development" conducted in FY2022. The present study aims to goal of this study is to implement a research plan relate to a development of combinational technology of new chemical analysis with informatics, and the aim is to develop new system for whole image estimation system using small quantities of information.

Journal Articles

Atomic position and the chemical state of an active Sn dopant for Sn-doped $$beta$$-Ga$$_{2}$$O$$_{3}$$(001)

Tsai, Y. H.*; Kobata, Masaaki; Fukuda, Tatsuo; Tanida, Hajime; Kobayashi, Toru; Yamashita, Yoshiyuki*

Applied Physics Letters, 124(11), p.112105_1 - 112105_5, 2024/03

JAEA Reports

Contribution to risk reduction in decommissioning works by the elucidation of basic property of radioactive microparticles (Contract Research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*

JAEA-Review 2023-021, 112 Pages, 2024/02

JAEA-Review-2023-021.pdf:7.1MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted from FY2018 to FY2021 (this contract was extended to FY2021). The present study aims to understand the basic properties (size, chemical composition, isotopic composition - including concentration of $$alpha$$-emitters, electrostatic properties, and optical properties, etc.) of fine particles composed of silicate with insoluble properties which contain regions of highly concentrated radioactive cesium (Cs) released to the environment by the accident at the Fukushima Daiichi Nuclear Power Station of TEPCO in 2011 March.

Journal Articles

An Analytical model to decompose mass transfer and chemical process contributions to molecular iodine release from aqueous phase under severe accident conditions

Zablackaite, G.; Shiotsu, Hiroyuki; Kido, Kentaro; Sugiyama, Tomoyuki

Nuclear Engineering and Technology, 56(2), p.536 - 545, 2024/02

 Times Cited Count:0

Journal Articles

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

Yamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

Journal Articles

Thermal conductivity measurement of uranium-plutonium mixed oxide doped with Nd/Sm as simulated fission products

Horii, Yuta; Hirooka, Shun; Uno, Hiroki*; Ogasawara, Masahiro*; Tamura, Tetsuya*; Yamada, Tadahisa*; Furusawa, Naoya*; Murakami, Tatsutoshi; Kato, Masato

Journal of Nuclear Materials, 588, p.154799_1 - 154799_20, 2024/01

 Times Cited Count:1 Percentile:72.91(Materials Science, Multidisciplinary)

The thermal conductivities of near-stoichiometric (U,Pu,Am)O$$_{2}$$ doped with Nd$$_{2}$$O$$_{3}$$/Sm$$_{2}$$O$$_{3}$$, which is major fission product (FP) generated by a uranium-plutonium mixed oxides (MOX) fuel irradiation, as simulated fission products are evaluated at 1073-1673 K. The thermal conductivities are calculated from the thermal diffusivities that are measured using the laser flash method. To evaluate the thermal conductivity from a homogeneity viewpoint of Nd/Sm cations in MOX, the specimens with different homogeneity of Nd/Sm are prepared using two kinds of powder made by ball-mill and fusion methods. A homogeneous Nd/Sm distribution decreases the thermal conductivity of MOX with increasing Nd/Sm content, whereas heterogeneous Nd/Sm has no influence. The effect of Nd/Sm on the thermal conductivity is studied using the classical phonon transport model (A+BT)$$^{-1}$$. The dependences of the coefficients A and B on the Nd/Sm content (C$$_{Nd}$$ and C$$_{Sm}$$, respectively) are evaluated as: A(mK/W)=1.70 $$times$$ 10$$^{-2}$$ + 0.93C$$_{Nd}$$ + 1.20C$$_{Sm}$$, B(m/W)=2.39 $$times$$ 10$$^{-4}$$.

Journal Articles

Nuclear data as foundation of nuclear research and development

Fukahori, Tokio; Nakayama, Shinsuke; Katabuchi, Tatsuya*; Shigyo, Nobuhiro*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 65(12), p.726 - 727, 2023/12

The Investigative Committee on Nuclear Data investigates and observes global trends in nuclear research and development and conducts comprehensive examinations of Japanese nuclear data activities from a broader perspective, as well as cooperation with domestic and foreign academic institutions in a wide range of fields other than the Atomic Energy Society. We aim to establish a system for communication, information exchange, and interdisciplinary cooperation. In this report, we will report on three of the main activities for the 2021-2022 term: a request list site for nuclear data, human resource development, and roadmap production.

Journal Articles

Understanding muon diffusion in perovskite oxides below room temperature based on harmonic transition state theory

Ito, Takashi; Higemoto, Wataru; Shimomura, Koichiro*

Physical Review B, 108(22), p.224301_1 - 224301_11, 2023/12

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

JAEA Reports

Effect of preparation conditions and storage time on characteristic and rheological properties of carbonate slurries

Kato, Tomoaki; Yamagishi, Isao

JAEA-Technology 2023-018, 53 Pages, 2023/11

JAEA-Technology-2023-018.pdf:2.6MB

In the decommissioning of Fukushima Daiichi Nuclear Power Station, radioactive carbonate slurry waste was generated using the Advanced Liquid Processing System (ALPS) pretreatment and temporarily stored in a high integrity container (HIC). In 2015, overflow of supernatant from HIC estimate as bubble retention in the carbonate slurry was discovered, increasing the need for a safety assessment of the carbonate slurry stored the HIC (HIC slurry). In this study, a carbonate slurry (simulated slurry) was prepared according to the Mg/Ca mass ratio in the ALPS inlet water of the HIC slurry which overflew the HIC. The effects of reaction time during the pretreatment process, suspended solids concentration (SS concentration), and settling time on the particle composition, morphology and rheological properties of the slurry were investigated. Evaluating the effect of reaction time and concentration process on chemical properties in slurry production, the effect of the reaction time was not confirmed in the simulated slurry that had undergone the concentration process, and slurry prepared at SS concentration of 150 g/L was composed of formless particles have a particle diameter of 0.4 $$mu$$m or less. We also investigate the effect of SS concentration on sedimentability, decrease in SS concentration by dilution with processing solution contributed to an increase in the initial slurry settling velocity. Furthermore, two different flow characteristics were observed depending on the settling time, suggesting that the slurry at the initial settling time has non-Bingham flow properties, whereas it changes to Bingham flow properties as the settling time becomes longer. In addition, yield stress was increased with settling time, and this yield stress was found to be exponentially proportional to the density of the slurry. These results provide knowledge to estimate the current state of HIC slurry and are expected to contribute to the safety assessment.

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities, 2

Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro

JAEA-Data/Code 2023-011, 32 Pages, 2023/11

JAEA-Data-Code-2023-011.pdf:0.93MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{235}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.

Journal Articles

Measurements of capture cross-section of $$^{93}$$Nb by activation method and half-life of $$^{94}$$Nb by mass analysis

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi

Journal of Nuclear Science and Technology, 60(11), p.1361 - 1371, 2023/11

 Times Cited Count:1 Percentile:72.91(Nuclear Science & Technology)

The thermal-neutron capture cross section ($$sigma$$$$_{0}$$) and resonance integral (I$$_{0}$$) for $$^{93}$$Nb among nuclides for decommissioning were measured by an activation method and the half-life of $$^{94}$$Nb by mass analysis. Niobium-93 samples were irradiated with a hydraulic conveyer installed in the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Gold-aluminum, cobalt-aluminum alloy wires were used to monitor thermal-neutron fluxes and epi-thermal Westcott's indexes at an irradiation position. A 25-$$mu$$m-thick gadolinium foil was used to sort out reactions ascribe to thermal-and epi-thermal neutrons. Its thickness provided a cut-off energy of 0.133 eV. In order to attenuate radioactivity of $$^{182}$$Ta due to impurities, the Nb samples were cooled for nearly 2 years. The induced radio activity in the monitors and Nb samples were measured by $$gamma$$-ray spectroscopy. In analysis based on Westcott's convention, the $$sigma$$$$_{0}$$ and I$$_{0}$$ values were derived as 1.11$$pm$$0.04 barn and 10.5$$pm$$0.6 barn, respectively. After the $$gamma$$-ray measurements, mass analysis was applied to the Nb sample to obtain the reaction rate. By combining data obtained by both $$gamma$$-ray spectroscopy and mass analysis, the half-life of $$^{94}$$Nb was derived as (2.00$$pm$$0.15)$$times$$10$$^{4}$$ years.

Journal Articles

Quantitative visualization of a radioactive plume with harmonizing gamma-ray imaging spectrometry and real-time atmospheric dispersion simulation based on 3D wind observation

Nagai, Haruyasu; Furuta, Yoshihiro*; Nakayama, Hiromasa; Satoh, Daiki

Journal of Nuclear Science and Technology, 60(11), p.1345 - 1360, 2023/11

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A novel monitoring method for the quantitative visualization of 3D distribution of a radioactive plume and source term estimation of released radionuclides is proposed and its feasibility is demonstrated by preliminary test. The proposed method is the combination of gamma-ray imaging spectroscopy with the Electron Tracking Compton Camera (ETCC) and real-time high-resolution atmospheric dispersion simulation based on 3D wind observation with Doppler lidar. The 3D distribution of a specific radionuclide in a target radioactive plume is inversely reconstructed from line gamma-ray images from each radionuclide by several ETCCs located around the target by harmonizing with the air concentration distribution pattern of the plume predicted by real-time atmospheric dispersion simulation. A prototype of the analysis method was developed, showing a sufficient performance in several test cases using hypothetical data generated by numerical simulations of atmospheric dispersion and radiation transport.

Journal Articles

Review of JENDL/HE-2007 neutron-induced fission cross sections of uranium-235 and 238 above 200 MeV

Fukahori, Tokio

INDC(JPN)-210 (Internet), 5 Pages, 2023/10

The $$^{235}$$U(n,f) cross section values were not correctly compiled in the ENDF format, and wrong values are disseminated in the JENDL/HE-2007 file. The high energy part of the $$^{235}$$U(n,f) cross section for the JENDL/HE-2007 library was evaluated by using the results of the FISCAL code. The correct $$^{235}$$U(n,f) cross section values of the JENDL/HE-2007 library above 200 MeV is given in this report.

Journal Articles

Molecular dynamics analysis of reactor graphite for preparing thermal neutron scattering law

Okita, Shoichiro; Goto, Minoru

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 10 Pages, 2023/10

Journal Articles

In situ transmission electron microscopy observation of melted germanium encapsulated in multilayer graphene

Suzuki, Seiya; Nemoto, Yoshihiro*; Shiiki, Natsumi*; Nakayama, Yoshiko*; Takeguchi, Masaki*

Annalen der Physik, 535(9), p.2300122_1 - 2300122_12, 2023/09

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

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